Yes, was my first thought from the time of your very first picture of that tank.. "Its an Angelfish tank." MADE for angels.
Well, its not that its really any better for them, its just that it would show them off so nicely. One thing you will always have to remember about your tank is that it can't be thought of in quite the same way as the large gallonage would have you think, since it has a small relative surface area. My own thought about that (completely uncscientific) is that the thing of going over "one inch per US gallon" guideline, say up to 1.5" or 2" later on with overfiltration, mature filters and good maintenance, should
not be done with this tank. My feeling is that it just would
not have enough oxygen due to the small surface area.
So as long as you stuck to the "one inch" guideline, and I vaguely remember angelfish as counting as 4 inches of fish body when mature, then you could work out a number. Personally, I like the idea of the "small" cory catfish as a bottom population. There are three types and two of the three will hang out at the bottom, while the third type will go mid tank. Either of the bottom types would be great with angelfish and they need to be in a little shoal of 5 or 6, but I think they only count as an inch or even less each. MW & OM47 are familiar with the types, but I'm sure they're listed with the cories, I'm just too lazy to look.
~~waterdrop~~