Welp, considering you're empty now, you may was well cycle out all the water, yes. 90 or 100% water change to get rid of what you added.
As far as a new CYCLE, like nitrogen cycle, no, you should be alright. Your biofilter should still be decently intact, so your options are to either go out and by a bunch of new fish, or start dosing ammonia so your bacteria doesnt die off.
Like you said, you live and learn. One of the things Ive learned from this forum is that it is better to keep fish in an adverse condition (high pH for a lower pH fish, etc) then it is to try to manufacture water chemistry changes, especially those pertaining to pH since most chemical compounds introduce rapid and often not very effective changes to pH.
What were you attempting to do with manually adjusting the pH? Anyhow, I'm sorry that you lost all your fish, but you've learned a valuable lesson in the process.
One redeeming this is that it is tons of fun to stock a tank, so cut your losses, grieve as you may, and get to stocking!
Best,
Ryan